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"Kinetics of Aquation of Pentaamminechlorocobalt(III) and Kinetics of Decomposition of Tetraamminecarbonatocobalt(III) Revisited. Synthesis, characterization, and determination of pKaof coordinated water in aquopentaamminecobalt(III) trichloride"
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"The hydrolysis of [Co(NH3)5Cl]2\u002Bin acidic solution follows a pseudo-first-order rate law , \uD835\uDC5F\uD835\uDC4E\uD835\uDC61\uD835\uDC52=\uD835\uDC58\u2032[\uD835\uDC34]\uD835\uDC5A, in which k\u2019=k[H2O]nand A = [Co(NH3)5Cl]2\u002B. The order m was found by the method of initial rates to be ~1. The observed rate constant found at 25\u00B0C, 4.17\u00D710-5s-1, was able to be compared to the literature value7of 1.72\u00D710-6s-1. This inconsistency is attributed to differences in ionic strength. The activation energy, Ea, was found to be 45 kJ/mol and the frequency factor, A, was found to be 3.8\u00D7103s-1. An enthalpy, \u0394H, of 94 kJ/mol matched appropriately with the accepted value of 93 kJ/mol. Additionally, the pKaof coordinated water in [Co(NH3)5(H2O)]Cl3could be determined using titration and spectroscopy. The titrimetric method yielded a pKaof 5.66, while the two spectroscopic methods gave pKa\u2019s of 5.96 and 5.77. An average pKaof 5.80 was determined, making the coordinated water ~10 billion times more acidic than uncoordinated water. Lastly, the kinetics of the decomposition of [Co(NH3)4(CO3)]NO3were studied.The reaction follows a rate law \uD835\uDC5F\uD835\uDC4E\uD835\uDC61\uD835\uDC52=\uD835\uDC58\u2032[(\uD835\uDC41\uD835\uDC3B3)4\uD835\uDC36\uD835\uDC5C\uD835\uDC36\uD835\uDC423\u002B]\uD835\uDC5A, wherek\u2019 = [H\u002B]nat a constant pH. The reaction was studied at three different pH\u2019s and the k\u2019 value determined for each. It was concluded that both m and n equal one, giving the reaction a second order rate law."
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"2016 January 25"
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"Schneider, Sarah",
"Ghosh, Phalguni",
"Middlesex College, Department of Natural Sciences"
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"Kinetics of Aquation of Pentaamminechlorocobalt(III) and Kinetics of Decomposition of Tetraamminecarbonatocobalt(III) Revisited. Synthesis, characterization, and determination of pKaof coordinated water in aquopentaamminecobalt(III) trichloride"
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